Finite element models of headforms are used in experimental simulations of pedestrian protection. In this study, a quick and accurate method for FE modeling of the headforms was developed. This method entailed the initial definition of the dimensional parameters for the mass, centroid, and inertial moment properties of the headform. The equations governing these properties were constructed using the dimensional parameters as design variables. The dimensional parameters meeting the requirements of the relevant regulations were obtained by solving these three equations. A design optimization model was constructed for the material parameters of the outer part of the headform. In this model, the parameters of the material used in the FE model were considered as design variables; the difference between the peak acceleration in a side-impact simulation test and the average value of the regulated acceleration range was used as the objective function; the first-order natural frequency, which was required to be greater than 5,000 Hz, was defined as one of the constraints; the peak drop acceleration, which was required to be within the regulated range of values, was defined as the second constraint. The material parameters were obtained by solving the optimization model. These material parameters meet the dynamic requirements of the regulations for headforms. Based on these three parameters, an FE model of a headform can be constructed quickly and accurately.