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Influence of defective sites in Pt/C catalysts on the anode of direct methanol fuel cell and their role in CO poisoning: a first-principles study
Soonchul Kwon, Seung Geol Lee 한국탄소학회 Carbon Letters 5 Pages
한국탄소학회 Carbon Letters 2015, Vol.16 No.3 6 198-202 (5 pages)
on electronic properties such as adsorption energy and electronic band gap. Interestingly, the presence of neighboring defect sites led to a reduction of H2 dissociation and CO poisoning due to atomic Pt filling the defect sites. At distant sites, H2 dissociation was active on Pt, but CO filled the defect sites to form carbon π-π bonds, thus enhancing the oxidation of the carbon surface. It should be noted that defect sites can cause CO poisoning, thereby deactivating the anode gradually. -
Photocatalytic degradation and antibacterial investigation of nano synthesized Ag₃VO₄ particles @PAN nanofibers
Prem Singh Saud, Zafar Khan Ghouri, Bishweshwar Pant, Taehee An, Joong Hee Lee, Mira Park, Hak-Yong Kim 한국탄소학회 Carbon Letters 7 Pages
한국탄소학회 Carbon Letters 2016, Vol.18 5 30-36 (7 pages)
methylene blue. Their structural, optical, and photocatalytic properties have been studied by X-ray diffraction, transmission electron microscopy, field-emission scanning electron microscopy equipped with rapid energy dispersive analysis of X-ray, photoluminescence, and ultraviolet?visible spectroscopy. The characterization procedures revealed that the obtained material is PAN nanofibers decorated by Ag₃VO₄ nanoparticles. Photocatalytic degradation of methylene blue investigated in an aqueous... -
One-step synthesis of dual-transition metal substitution on ionic liquid based N-doped mesoporous carbon for oxygen reduction reaction
Ulziidelger Byambasuren, Yukwon Jeon, Dorjgotov Altansukh, Yunseong Ji, Yong-Gun Shul 한국탄소학회 Carbon Letters 12 Pages
한국탄소학회 Carbon Letters 2016, Vol.17 No.1 8 53-64 (12 pages)
ionic liquid (3-methyl-1-butylpyridine dicyanamide) for N/C species and a mesoporous silica template for the physical structure. Mostly, N-doped carbons are promoted by a single transition metal to improve catalytic activity for ORR in PEMFCs. In this study, our N-doped mesoporous carbons were promoted by the dual transition metals of iron and cobalt (Fe, Co), which were incorporated into the N-doped carbons lattice by subsequently heat treatments. All the prepared carbons were characterized by...
