Present study visualized flow pattern and investigated spray characteristics of twin-fluid atomization with converging-diverging nozzles. Particle sizes were measured by using the Malvern particle analyzer, and the radial size distributions were evaluated by using the tomographic transform technique. The results show that the SMD generally increases in the radial direction at a prescribed liquid flow rate and the increasing rate in the SMD becomes gradual as atomizing gas pressure increases. The SMD decreases as the liquid flow rate increases at a fixed GLR (gas/liquid mass ratio). The atomization performance of the protrusion-type nozzle turned out to be superior to that of the flush-type. However, in the case of the protrusion-type, flow separation occurs outside the liquid delivery tube when the pressure at the gas nozzle chamber is high enough, which may deteriorate the atomization performance.