The higher order harmonic components of magnetostriction during ac magnetization in 3% SiFe are measured as a function of the magnetizing angle respect to [001] axis using a constructed laser interferometry. The magnetostriction with magnetizing angle from [001] axis agrees ith the calculation based on domain reorientation. The relative amplitudes of odd and even harmonics respectively for magnetic induction and magnetostriction decrease with the order of harmonics, accompanying the contraction of the amplitudes. The contraction of harmonics order of magnetostriction harmonics is shown to be the even number times of that of magnetic induction.