This paper documents the effect of surface treatment of aluminum on the bonding strength of aluminum/CFRP composites. The surface of aluminum panel was treated by DC plasma. The optimal treatment condition of the aluminum was determined by measuring the contact angle and T-peel strength as functions of mixture ratio of acetylene gas to nitrogen gas. The mixture ratios used were 1:9, 3:7, 5:5, 7:3, and 9:1 Lap shear tests and T-peel tests were performed using surface-treated alumiunm/CFRP composites and regular alumiunm/CFRP composites. The results showed that the contact angle was minimized and the T-peel strength was maximized iota the mixture ratio of 5:5. The results also showed that the shear strength of surface-treated alumiunm/CFRP composites was 34% greater than that of regular alumiunm/CFRP composites. The T-peel strength of surface-treated alumiunm/CFRP composites was also 5 times greater than that of regular alumiunm/CFRP composites.