Observing of GMT-Sheet in molding conditions, we have investigated unexpected phenomenons of moldings surface. In microscope investigation, we observe that there exist deficiencies on the surface of GMT-Sheet moldings, such as the spherulite, fiber projection, crack, fiber exposure, micro-weldline, pinhole and winding. They are caused to arise unevenness and phenomenons influence polish on surface. Especially, the major cause of the unevenness, effected to surface roughness, is a shrinking of matrix in the process of holding pressure and cooling temperature. The higher holding pressure load in a molding process and the lower demolding temperature in an annealing experiment, the better GMT-Sheet moldings improved its appearance.