In power cables as one of the important power applications adopting HTS tapes, a good insulation should be kept at its optimum performance. As an insulation material for superconducting device applications, polypropylene laminated paper (PPLP) is now widely used instead of the conventional Kraft paper. In addition to its dielectric property, the insulation material should also possess superior mechanical property at cryogenic temperatures and operability that is necessary for the insulation winding process. This study aims to evaluate the mechanical property of the PPLP material at ambient and cryogenic temperatures. At cryogenic temperature, the failure stress of PPLP increased significantly as compared with that at ambient temperature. The failure stress at both temperatures depended upon the sample orientation to the load application.