The present paper discusses the characteristics of unsteady aerodynamic forces on long-span curved roofs. A forced vibration test is carried out in a wind tunnel to investigate the effects of wind speed, vibration amplitude, reduced frequency of vibration and rise/span ratio of the roof on the unsteady aerodynamic forces. Because the range of parameters tested in the wind tunnel experiment is limited, a CFD simulation is also made for evaluating the characteristics of unsteady aerodynamic forces on the vibrating roof over a wider range of parameters. Special attention is paid to the effect of reduced frequency of vibration. Based on the results of the wind tunnel experiment and CFD simulation, the influence of the unsteady aerodynamic forces on the dynamic response of a full-scale long-span curved roof is investigated on the basis of the spectral analysis.