In order to study gross alpha analysis method using LSC, the efficiency tests with uranium standard materials were performed and then compared with the GPC method (US EPA 900.0 method) using 15 groundwater samples. For 15 groundwater samples, the average efficiencies of the GPC and LSC method were 7~11% and 90%, respectively. The average precisions of the GPC and LSC method were 16.16% and 6.00%, respectively. Also, The average standard deviations for 15 samples were 7.38 pCi/L and 2.95 pCi/L, respectively. The determination coefficient of the tested results by two methods was 0.9948. As a result, the LSC method tested in this study was applicable for the screening of the gross alpha and showed the advantages in the gross alpha measurement due to the simple measurement procedures.